It may be possible to have a demonstration experiment that shows the absorptive properties of CO2 but not as described. Nothing so simple -
It is important to consider that the greenhouse effect works within a depth of atmosphere from sea level to low to mid stratosphere, ie much greater distance than 3m (up to 20,000m)- albeit with declining density and effect as the altitude rises. The rate of current warming averages around 0.2 C per decade, with periods of 3 decades preferred to avoid misconstruing natural climate variability for a trend. That is not conducive to hour to hour or day to day or even year to year measurement; averaging of highly varying temperatures over a sufficient time that a longer term trend can be determined is required.
I think John Tyndall's equipment for testing the radiant heat absorption of gases including CO2 - that, as a consequence of explaining how Earth's average temperature could be what it was, laid the groundwork for understanding that human activities, especially fossil fuel burning could change it - does look the part -